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I think this will all end if she has a child and love that child.. i think thats when the whole "love" thing becomes a concrete idea. I think Raymond loved her enough the whole 100 years so just his "love" wouldnt be the answer.
Then the curse will be transferred to her child. I really think the going back time loop is a curse atp.. and i think its heridetary unless their heir is fully capable of loving their partner and building their own family.
I think the author of the novel they're in is sick if that was the case. Imagine forcing the characters to realise his own concept of "love" instead of giving them free will. What if the characters want to be single for life? You'd keep them looping till they force themselves to fall in love? Sick.